Suarez won the LaLiga title with Atletico under Simeone after being forced out of Barcelona.
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Now with Inter Miami, the veteran striker said on Simplemente Fútbol: "He was a coach who taught me a lot.
"You can discuss some issues with him, exchange opinions, but he helped me a lot to find my rhythm and overcome that weakness that led me to show that I was still up to the task. It was a spectacular year.
"The coach and all my teammates helped me a lot at Atlético to win a title after so many years."